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nanoparticles and applications in super-resolution imaging
With the rapid development of social science and technology, optical microscopes have gone through the development process of ordinary optical microscopes with limited diffraction to the fluorescence super-resolution microscopes that break the diffraction limit, as well as non-fluorescent, label-free super-resolution optical microscopes. The non-fluorescent super-resolution imaging based on the nonlinear scattering of plasmonic nanoparticles is an interesting research topic and has been successfully applied to the imaging of biological cells. However, it has been found in the research that gold nanoparticles have severe overheating problems, aggregation and coupling between nanoparticles are prone to occur, and high temperature melting at high laser power is likely to affect practical applications.
The photothermal effect of nanoparticles is closely related to the thermal conductivity of the surrounding medium. Therefore, it is of great significance to study the key role of local thermal environment in the nonlinear scattering of plasmonic nanoparticles, and to further develop the label-free super-resolution imaging.
Recently, the research group led by Prof. Xiangping Li at Jinan University (JNU) proposed the strategy of Au@SiO2 core-shell particles, in order to improve the above-mentioned shortcomings of gold nanoparticles, and studied the mechanism of the nonlinear scattering saturation of gold nanoparticles based on the photothermal effect, and they also explored the application of Au@SiO2 in super-resolution imaging. Benefitting from the enhanced thermal stability and the reduced plasmonic coupling provided by the shell-isolated nanoparticles, the super-resolution imaging with a feature size of 52 nm (λ/10) can be achieved, and pairs of nanoparticles with a gap-to-gap distance of 5 nm can be readily resolved. This work was published in Chinese Optics Letters 2023, Vol. 21, No. 10 Tianyue Zhang, Zhiyuan Wang, Xiangchao Zhong, Ying Che, Xiangping Li. Photothermal nonlinear scattering of shell-isolated gold nanoparticles and applications in super-resolution imaging[J]. Chinese Optics Letters, 2023, 21(10): 103601) and was selected as the cover of the issue.
Principle: Gold nanoparticles are irradiated by incident light field, resulting in the temperature rising due to the photothermal effect. When the temperature reaches a certain threshold, the permittivity of the gold material is no longer constant, but instead becomes dependent on the temperature changes, leading to the nonlinear relationship between the temperature elevation and the excitation intensity. In turn, the change of optical constant of the material will further affect the plasmonic resonance of the particle, and consequently induces the scattering modulation. The optical super-resolution imaging of gold nanoparticles based on saturation scattering properties is realized by using the point spread function modulation technique of suppressed scattering imaging (SUSI) microscope.
Figure 1 (a) Illustration of optical heating of the gold nanospheres that converts light into temperature rises. Due to the difference in the local thermal media, the gold nanospheres (top: in immersion oil, middle: in SOG materials, and bottom: with silica coatings) undergo various temperature rising. (b) Experimental measurements of nonlinear plasmonic scattering of the five prepared samples, showing the nonlinear dependency of scattering on irradiance intensities for CW excitations at the wavelength of 532 nm. (c)The gap-to-gap distances of two nanoparticles are shown in the SEM images. The super-resolution imaging of the shell-isolated nanoparticles clearly shows the resolving ability to distinguish two nanoparticles that are closely located in sub-diffraction spaces as small as 5 nm.
The photothermal nonlinear scattering efficiency of gold nanoparticles is related to the thermal conductivity of the local environment related to heat dissipation. Five different samples were prepared with 70 nm diameter gold nanospheres immersed in oil, coated with silica shells with various thicknesses (shell thickness of 10 nm, 23 nm and 40 nm, respectively), and encapsulated in spin-on glass (SOG) material. To this extent, the gold spheres in all cases are in the same optical environment due to the homogenous medium dielectric constant, but they experience different local thermal environments caused by varied immediate surroundings during optical heating. The experimental results have proved that the local heat dissipation of the particles can be effectively improved by coating the SiO2 layer, therefore reduce the heat accumulation, and avoid the melting of gold cores. Compared with the bare gold nanospheres, the shell-isolated gold nanoparticles are not only photothermally more stable but also can effectively prevent plasmon coupling due to particle aggregations. This enables us to access the super resolving of two individual shell-isolated nanoparticles with the gap-to-gap distance
of 5 nm. The full-width at half-maximum (FWHM) of the measured image spot from the single core-shell nanoparticle (70 nm gold core with 40 nm silica shell) can be squeezed to 52 nm (∼λ/10).
The JNU researchers believe that the proposed method of using shell-isolated gold nanoparticles with a silica coating for photothermal nonlinear scattering represents a new principle and technology for non-fluorescence super-resolution imaging. It has potentials to be applied to the imaging of microscopic structures such as cells and tissues, which is helpful to the study of biological processes and the pathogenesis of diseases.
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Recently, topological charge, which can act as a measure of the angular momentum of vortex beams, has been established as a robust information carrier that is capable of being transmitted over numerous kilometers without any free-space path loss. It suggests that this technology is ready for operational deployment. However, as communication links are further extended to accommodate it, turbulence accumulated during propagation will result in the transmitted orbital angular momentum (OAM) signals becoming severely distorted, even under conditions of relatively weak turbulence. Apart from familiar turbulence effects such as beam wander, beam spreading and scintillation, it will also be important to take into account vortex splitting effects, which affect the precision of OAM signal reception. Vortex splitting refers to the topological charge of vortex beams breaking up where l >1 to give l individual single-charge vortices. These vortices cross the transverse plane quasi-independently. Generally, the larger the vortex splitting ratio, the smaller the average OAM value that can be measured.
The research group led by Prof. Lixin Guo from Xidian University, propose a new method to mitigate vortex splitting in free-space optical communication by using the self-healing effect of auto-focusing Airy vortex beams (AAVB). The value of this work is that two common modes of coupling autofocusing Airy beams with vortices are unified by introducing a parameter that controls the AAVB intensity gradients. Through the action of self-healing effect, the energy of optic field flows inward radially, trapping the individual vortices. For this to be effective, the right intensity gradients need to be selected for different degrees of turbulence, thus improving the accuracy of OAM reception. The results of this work have been published in Chinese Optics Letters, Vol 17, Issue 4, 2019 (Xu Yan, et al. Free-space propagation of autofocusing Airy vortex beams with controllable intensity gradients).
“This is a very valuable study that realizes the simultaneous modulation of beam trajectory and focus intensity without destroying the original AAVB structure, providing an effective new way of reducing vortex splitting” said Prof. Guo.
For now, the research regarding vortex beam propagation is still focused on weak turbulence conditions. The realization of effective transmission and reception of OAM signals under conditions of strong turbulence and scattering media will be the focus of the group’s future work.
Fig. 1. (a)-(d) Intensity distributions of AAVBs with l = 3 for different values of m = 0, 1.6, 3.0, and 5.0 after propagation through a turbulent optical channel. (e)-(h) Phase cross-sections of AAVBs corresponding to (a)-(d), respectively.
- Apr. 22, 2019
- Vol. 17, Issue 4 (2019)
With the rapid growth of the data traffic for hyper-scale internet data centre, the demand for high speed optical transceiver modules to interconnect among the intra and inter data centres beyond 100 Gbit/s becomes strong. Due to the limited space of the high port density line card data network center, the optical transceivers modules with small form factor are required to increase port density of line cards in communication systems. Considering the maturity of the process, the hybrid integration technology that assemble various discrete components in an ultra-compact tube is proposed to ensure the yield of the device.
For packaging process of receiver optical subassembly (ROSA) modules, the microwave circuit usually contains two parts of a radio frequency circuit and a bias network on which many capacitors and resistors are mounted. If they are all installed in one circuit board, it will easily cause crosstalk and distortion of the electrical signals. To overcome this drawback, the research group led by Dr. Jianguo Liu from Institute of Semiconductors, Chinese Academy of Sciences, proposed a 3D microwave circuit which allows radio frequency (RF) signal and bias voltage to be isolated in physical space for compact packaging. The value of this work is the experimental three-dimensional assembly of the ultra-compact ROSA based on the high speed microwave modeling. The -3 dB bandwidths of four channels of the fabricated module are all up to 20 GHz and the frequency response results are in very good agreement between the modeling and the experimental measurements. The results will extend our knowledge on hybrid-integrated technology. This work entitled Ultra-compact four-lane hybrid-integrated ROSA based on three-dimensional microwave circuit design has been published in Chinese Optics Letters, Vol. 17, Issue 3, 2019.
“The module used not only for 4×25 Gb/s non-return to zero (NRZ) modulation transmission, but also for many RF transmission systems such as remote antennas, satellite antennas, and secure encrypted communication. In addition, it can also be applied to radar systems to achieve full-band detection of radar”said Dr. Jianguo Liu from the research group.
With the multi-faceted application of detectors in radio-over-fiber (ROF) systems and digital center systems, detector modules will move toward high power output, high signal-to-noise ratio, miniaturization, integration, and low power consumption. The further work will focus on the integration of detector chips with other functional chips, such as semiconductor optical amplifier (SOA) chips, trans-impedance amplifier (TIA) chips, and development of multi-function devices.
The internal detailed configuration of the ROSA.
- Mar. 12, 2019
- Vol. 17, Issue 3 (2019)
High-precision measurement of absolute gravity is very important in Geophysics, Geodesy, Hydrology, Seismology, etc. It is difficult to evaluate the accuracy of an absolute gravimeter (AG) by itself, since the local absolute gravity value is always changing with time and position. Therefore, the comparison between different high-precision absolute gravimeters is of great importance for the evaluation of the instrument accuracy.
Researchers from Zhejiang University of Technology and Zhejiang University reported their compact cold atom gravimeter (CCAG) for participating in the first Asia-Pacific Comparison of Absolute Gravimeters (APMP.M.G-K1), which was the first CCAG participating in a Regional Absolute Gravity Comparison in China. The principle of the CCAG is based on the matter wave interference. The test mass in the CCAG is the microcosmic atoms rather than the classic object, which makes the CCAG more suitable for the continuous gravity monitoring. The accuracy of this gravimeter was evaluated to be about 19 μGal after the correction of the main systematic errors. The sensitivity was estimated to be 90 without any vibration isolation system during measurement. This work has been published in Chinese Optics Letters, Volume 17, Issue 1, 2019 (Zhijie Fu, et al., Participation in the absolute gravity comparison with a compact cold atom gravimeter).
Professor Qiang Lin, director of the group, believes that there are still spaces to improve the absolute accuracy of the CCAG. The successful participation and measurement of the CCAG in the APMP.M.G-K1 provides valuable experiences for the improvement of this kind of gravimeter.
Based on the comparison results, further work will be focused on the improvement of accuracy and the suppression of systematic noises.
A compact cold atom gravimeter participating in the Comparison of Absolute Gravimeters.
- Mar. 11, 2019
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Chinese Optics Letters (COL) invites high-quality articles for the Special Issue on the 20th anniversary of Wuhan National Laboratory for Optoelectronics (WNLO) to be published in Dec. 2023.
On the occasion of the 20th anniversary of the founding of COL, the WNLO has also gone through 20 years. The WNLO is one of the six national research centers approved by the Ministry of Science and Technology of China in 2017. Its predecessor was the Wuhan National Laboratory for Optoelectronics (preparatory), one of the five national laboratories approved for preparatory construction by the Ministry of Science and Technology of China in November 2003. The WNLO is jointly built by the Ministry of Science and Technology of China, Ministry of Education of China, Hubei Provincial Government, and Wuhan Municipal Government. It is supported by Huazhong University of Science and Technology, and there are three other joint organizations, namely Innovation Academy for Precision Measurement Science and Technology, CAS, China Information and Communication Technology Group Co., Ltd., and Huazhong Institute of Electro-Optics. The WNLO strives to become an academic innovation center, discipline leading center, talent cultivation center, scientific knowledge dissemination and achievement transfer center with important international influence in the field of optoelectronic science. As an interdisciplinary research center, the WNLO focuses on fundamental scientific and technological issues in the fields of information optoelectronics, energy optoelectronics, and life optoelectronics. After 20 years of development, it has achieved fruitful results in many fields including brain imaging, solar cells, ultra-fast lasers, laser manufacturing, optoelectronic devices and integration, data storage, etc.
This Special Issue plans to organize relevant experts to summarize the latest scientific research achievements and look forward to future trends in the fields of optoelectronics for information, energy and life science. Invited review articles and original research papers in these fields are welcome. All manuscripts will be subject to the normal standards and peer-review processes of this journal. These articles will help expand our communication and collaboration with colleagues, experts, and scholars from all over the world to better serve the optoelectronics community. Specific areas of interest include, but are not limited to:
● Optoelectronic devices and integration
● Multi-dimensional light field manipulation
● Optoelectronic information storage
● Ultra-strong and ultra-fast laser sources
● Laser manufacturing
● Photonics for energy
● Biomedical photonics
● Medical imaging
Guest Editor:
Jian Wang, jwang@hust.edu.cn
Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, China
Submission deadline: Aug 31st, 2023
Submission format:
Authors should use MS Word or LaTex style files. Please visit: Author Style Guide & Templates for the submission template and upload the submission on the following website: https://mc03.manuscriptcentral.com/clp-col under the type of "Special Issue on the 20th Anniversary of Wuhan National Laboratory for Optoelectronics (WNLO)".
- Aug. 17, 2023
- Vol. , Issue (2023)
Chinese Optics Letters (COL) invites high-quality articles for the Special Issue on the OISE major jointly established by Tianjin University and Nankai University to be published in Nov. 2023.
On the occasion of the 20th anniversary of the founding of COL, the Optoelectronic Information Science and Engineering (OISE) major jointly established by Tianjin University and Nankai University has also reached this milestone. Based on the guidance of the Ministry of Education (MoE) with the philosophy of independent education and close cooperation between the two universities, full use has been made of their advanced teaching, scientific research, and experimental bases and related resources, complementing each other's advantages, jointly establishing the major of "Optoelectronic Technology Science," and recruiting students from throughout the country since 2003. In 2012, the MoE uniformly adjusted the professional name to "Optoelectronic Information Science and Engineering." After 20 years of development, the major has produced more than 1000 high-level talents in the field of optical engineering and is engaged in research in many related fields.
The Special Issue plans to organize relevant experts to summarize the latest scientific research achievements in various fields over the past 20 years. It is hoped that these articles will help expand our communication and collaboration with colleagues, experts, and friends from all over the world to better serve the international optical community. This Special Issue is intended to invite experts and peers to outline the research progress or trends of optics, laser, and related hot topics or to contribute research papers (Invitation Only). All manuscripts must present original, previously-unpublished work and will be subject to the normal standards and peer-review processes of this journal. Specific areas of interest include, but are not limited to:
● Laser and nonlinear optics
● Optical sensing
● Micro and nano photonics
● Optical measurement and detection
● Terahertz technology
● Fiber optics
● Quantum optics
● Biomedical optics
● Optical information processing
Guest Editors:
Zhen Tian, tianzhen@tju.edu.cn
Tianjin University, China
Fei Fan, fanfei@nankai.edu.cn
Nankai University, China
Minglie Hu, huminglie@tju.edu.cn
Tianjin University, China
Weiwei Liu, liuweiwei@nankai.edu.cn
Nankai University, China
Submission deadline: July 31,2023
Submission format:
Authors should use MS Word or LaTex style files. Please visit: Author Style Guide & Templates for the submission template and upload the submission on the following website: https://mc03.manuscriptcentral.com/clp-col under the type of "Special Issue on OISE major jointly established by Tianjin University and Nankai University."
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- Oct. 14, 2020
- Vol. 19, Issue 6 (2020)
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- Feb. 06, 2020
- Vol. 18, Issue 8 (2020)
Submission Deadline: July 15, 2019
Chinese Optics Letters (COL) invites original manuscript submissions for a Special Issue on Underwater Wireless Optical Communication to be published in October 2019. The oceans, where life itself arose from, are a critical player in the basic elements indispensable for human life, like climate, weather, nourishment, and mineral resources, to name a few. For this reason, ocean exploration owns scientific, strategic and economic significance and has been attracting global attention. Foreseeing the rapid development of underwater exploration, a high-speed underwater wireless communication system becomes indispensable. Recently, underwater wireless optical communication (UWOC) has gained a renewed interest from both academic and industrial communities, because of its high bandwidth, compact antennas, low latency, cost-effectiveness and low power consumption. We envision many situations where the wireless optical links can be complementary to or even more competitive than its acoustic counterpart, such as broadband communications between various underwater vehicles and underwater sensors. By leveraging the low-absorption window of seawater in the blue-green band, optical signals can transmit several tens or hundreds of meters in general waters. In addition, an underwater optical wireless communication network can be implemented based on these optical links, to further enhance the transmission range, flexibility and robustness by virtue of multiple hops, and reliable network operation. The UWOC paves a new way to construct next-generation high-performance underwater wireless links in the immediate future.
The scope of this special issue covers all aspects of theoretical and experimental research related to UWOC. Specific areas of interest in UWOC include, but not limited to:
- Transmitter and receiver device, module and systems
- LED and laser based underwater optical links
- Channel characterization and modeling
- Narrow beam line-of-sight optical communications
- Non-line-of-sight communication links
- Self-powered underwater optical communication systems
- Networking and security issues
- Signal processing, etc.
Guest Editors:
Prof. Jing Xu, Zhejiang University
Email: jxu-optics@zju.edu.cn
Prof. Boon S. Ooi, King Abdullah University of Science & Technology
Email: boon.ooi@kaust.edu.sa
Prof. Gong-Ru Lin, Taiwan University
Email: grlin@ntu.edu.tw
The review process will be arranged for each submission individually, normally within 5 days after receiving the submission. The paper will be published online within one month after it is accepted.
Submission format: Authors should use the MS-Word or Latex style files. Please visit: Author Style Guide & Templates for the submission template and upload the submission at the website: https://mc03.manuscriptcentral.com/clp-col with the type of “Special issue on Underwater Wireless Optical Communication”.
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