• Photonics Research
  • Vol. 7, Issue 12, 1493 (2019)
Mi He1, Yequan Chen2, Lipeng Zhu3, Huan Wang1..., Xuefeng Wang2,4,*, Xinlong Xu1 and Zhanyu Ren1,5,*|Show fewer author(s)
Author Affiliations
  • 1Shaanxi Joint Laboratory of Graphene, State Key Laboratory Incubation Base of Photoelectric Technology and Functional Materials, International Collaborative Center on Photoelectric Technology and Nano Functional Materials, Institute of Photonics & Photon-Technology, Northwest University, Xi’an 710069, China
  • 2National Laboratory of Solid State Microstructures, Collaborative Innovation Center of Advanced Microstructures, School of Electronic Science and Engineering, Nanjing University, Nanjing 210093, China
  • 3School of Electronic Engineering, Xi’an University of Posts and Telecommunications, Xi’an 710121, China
  • 4e-mail: xfwang@nju.edu.cn
  • 5e-mail: rzy@nwu.edu.cn
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    DOI: 10.1364/PRJ.7.001493 Cite this Article Set citation alerts
    Mi He, Yequan Chen, Lipeng Zhu, Huan Wang, Xuefeng Wang, Xinlong Xu, Zhanyu Ren, "Third-order nonlinear optical properties of WTe2 films synthesized by pulsed laser deposition," Photonics Res. 7, 1493 (2019) Copy Citation Text show less

    Abstract

    The prominent third-order nonlinear optical properties of WTe2 films are studied through the Z-scan technique using a femtosecond pulsed laser at 1030 nm. Open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed at different intensities to investigate the nonlinear absorption and refraction properties of WTe2 films. OA Z-scan results show that WTe2 films always hold a saturable absorption characteristic without transition to reverse saturable absorption. Further, a large nonlinear absorption coefficient β is determined to be 3.37×103cm/GW by fitting the OA Z-scan curve at the peak intensity of 15.603GW/cm2. In addition, through the slow saturation absorption model, the ground state absorption cross section, excited state absorption cross section, and absorber’s density were found to be 1.4938×1016cm2, 1.2536×1016cm2, and 6.2396×1020cm3, respectively. CA Z-scan results exhibit a classic peak–valley shape of the CA Z-scan signal, which reveals a self-defocusing optical effect of WTe2 films under the measured environment. Furthermore, a considerable nonlinear refractive index value n2 can be obtained at 1.629×102cm2/GW. Ultimately, the values of the real and imaginary parts of the third-order nonlinear s
    T(z)=m=0(βI0Leff1+z2/z02)m(m+1)3/2,(1)

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    T=[1α(I)L]/(1α0L),(2)

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    α(I)=α01+I/IS+βI,(3)

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    T(L)=T0+TFN(L)T01T0(TmaxT0),(4)

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    TFN=ln{1+T0[eσgsE(0)1]}/σgsE(0),(5)

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    T(z)=14ΔΦ0(z/z0)(z2/z02+1)(z2/z02+9),(6)

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    Imχ(3)(esu)=c2n02β(m/W)/240π2ω,(7)

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    Reχ(3)(esu)=cn02n2(m2/W)/120π2,(8)

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    Mi He, Yequan Chen, Lipeng Zhu, Huan Wang, Xuefeng Wang, Xinlong Xu, Zhanyu Ren, "Third-order nonlinear optical properties of WTe2 films synthesized by pulsed laser deposition," Photonics Res. 7, 1493 (2019)
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