• Nano-Micro Letters
  • Vol. 16, Issue 1, 207 (2024)
Meiting Huang1, Mei Wang1, Liming Yang1,*, Zhihao Wang1..., Haoxuan Yu1, Kechun Chen1, Fei Han1, Liang Chen2,**, Chenxi Xu3, Lihua Wang2,4, Penghui Shao1 and Xubiao Luo1,4,***|Show fewer author(s)
Author Affiliations
  • 1National–Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization, Nanchang Hangkong University, Nanchang 330063, People’s Republic of China
  • 2Key Laboratory of Hunan Province for Advanced Carbon–based Functional Materials, School of Chemistry and Chemical Engineering,, Hunan Institute of Science and Technology, Yueyang 414006, People’s Republic of China
  • 3College of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, People’s Republic of China
  • 4School of Life Science, Jinggangshan University, Ji’an 343009, People’s Republic of China
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    DOI: 10.1007/s40820-024-01434-0 Cite this Article
    Meiting Huang, Mei Wang, Liming Yang, Zhihao Wang, Haoxuan Yu, Kechun Chen, Fei Han, Liang Chen, Chenxi Xu, Lihua Wang, Penghui Shao, Xubiao Luo. Direct Regeneration of Spent Lithium-Ion Battery Cathodes: From Theoretical Study to Production Practice[J]. Nano-Micro Letters, 2024, 16(1): 207 Copy Citation Text show less

    Abstract

    Direct regeneration method has been widely concerned by researchers in the field of battery recycling because of its advantages of in situ regeneration, short process and less pollutant emission. In this review, we firstly analyze the primary causes for the failure of three representative battery cathodes (lithium iron phosphate, layered lithium transition metal oxide and lithium cobalt oxide), targeting at illustrating their underlying regeneration mechanism and applicability. Efficient stripping of material from the collector to obtain pure cathode material has become a first challenge in recycling, for which we report several pretreatment methods currently available for subsequent regeneration processes. We review and discuss emphatically the research progress of five direct regeneration methods, including solid-state sintering, hydrothermal, eutectic molten salt, electrochemical and chemical lithiation methods. Finally, the application of direct regeneration technology in production practice is introduced, the problems exposed at the early stage of the industrialization of direct regeneration technology are revealed, and the prospect of future large-scale commercial production is proposed. It is hoped that this review will give readers a comprehensive and basic understanding of direct regeneration methods for used lithium-ion batteries and promote the industrial application of direct regeneration technology.
    Meiting Huang, Mei Wang, Liming Yang, Zhihao Wang, Haoxuan Yu, Kechun Chen, Fei Han, Liang Chen, Chenxi Xu, Lihua Wang, Penghui Shao, Xubiao Luo. Direct Regeneration of Spent Lithium-Ion Battery Cathodes: From Theoretical Study to Production Practice[J]. Nano-Micro Letters, 2024, 16(1): 207
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