• Ultrafast Science
  • Vol. 3, Issue 1, 0045 (2023)
Yudong Chen1,†, Zongyuan Fu1,†, Baochang Li2, Sainan Peng1..., Bingbing Zhu1, Guangyu Fan3, Yi Liu3, Chengyuan Ding4, Cheng Jin2,5 and Zhensheng Tao1,*|Show fewer author(s)
Author Affiliations
  • 1State Key Laboratory of Surface Physics, Key Laboratory of Micro and Nano Photonic Structures (MOE), and Department of Physics, Fudan University, Shanghai 200433, China.
  • 2Department of Applied Physics, Nanjing University of Science and Technology, Nanjing, Jiangsu 210094, China.
  • 3Shanghai Key Lab of Modern Optical System, University of Shanghai for Science and Technology, Shanghai 200093, China.
  • 4Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, China.
  • 5MIIT Key Laboratory of Semiconductor Microstructure and Quantum Sensing, Nanjing University of Science and Technology, Nanjing, Jiangsu 210094, China.
  • show less
    DOI: 10.34133/ultrafastscience.0045 Cite this Article
    Yudong Chen, Zongyuan Fu, Baochang Li, Sainan Peng, Bingbing Zhu, Guangyu Fan, Yi Liu, Chengyuan Ding, Cheng Jin, Zhensheng Tao. Phase-Matched High-Harmonic Generation under Nonadiabatic Conditions: Model and Experiment[J]. Ultrafast Science, 2023, 3(1): 0045 Copy Citation Text show less

    Abstract

    Nonadiabatic phase matching of high-harmonic generation (HHG) driven by few-cycle laser pulses is essential for extending harmonic energy and generating isolated attosecond pulses. However, understanding nonadiabatic HHG is challenging due to the complex interplay of various optical phases driven by temporally and spatially varying laser fields. Theoretical calculations typically rely on computationally demanding 3-dimensional simulations, which can make it difficult to extract the essential features of nonadiabatic HHG. In this work, we develop a computationally efficient 2-dimensional model that directly considers various phase contributions of HHG. Our model can well explain the experimentally observed pressure- and intensity-dependent behaviors of different harmonic orders. By appropriately parameterizing the single-atom response, our model can also estimate the variation of HHG spectra under different driving conditions. Our model can provide an efficient tool for the design and optimization of HHG-based applications.
    Yudong Chen, Zongyuan Fu, Baochang Li, Sainan Peng, Bingbing Zhu, Guangyu Fan, Yi Liu, Chengyuan Ding, Cheng Jin, Zhensheng Tao. Phase-Matched High-Harmonic Generation under Nonadiabatic Conditions: Model and Experiment[J]. Ultrafast Science, 2023, 3(1): 0045
    Download Citation